Researchers in France and Germany have created the first all-optical photonic time crystal. The nanostructure could be used to make ultrafast optical computers and amplifiers, frequency converters and perhaps even new types of lasers that work in the terahertz range.

Photonic crystals are nanostructured materials with a refractive index that varies on a length scale comparable to the wavelength of light, producing a phenomenon known as a photonic bandgap. This gap affects how photons propagate through the material in a way that resembles how a periodic potential in semiconductors affects the flow of electrons by defining allowed and forbidden energy bands. In the case of photonic crystals, light in certain wavelength ranges can pass through the material, but other wavelengths cannot.

Photonic time crystals (PhTCs) are similar to this, except their properties vary periodically in time, not space. Among other adjustments, this means that instead of photonic bandgaps, they host momentum bandgaps. These gaps are special in that light waves whose momenta fall within them grow exponentially in time.

Optical modulation at THz frequencies

PhTCs show much promise for applications like new types of tuneable lasers and ultrafast frequency converters, but controlling their photonic properties has proven very difficult. This is because these properties need to be modulated very strongly and on ultrashort timescales – on the order of the temporal period of the light itself.

Producing such extremely fast modulations is a key goal for scientists working in a branch of highly nonlinear optics known as time-domain photonics. Previously, their efforts have paid off in the microwave frequency range using PhTCs containing electrical circuits, but all-optical systems have proven elusive.

A team of physicists led by Yannis Laplace of the Ecole Polytechnique in France has now made a PhTC with properties that can be optically modulated at terahertz (THz, 10¹² Hz) frequencies. The new PhTC is made from a type of photonic crystal known as a plasmonic metamaterial: an artificially engineered nanostructure consisting of micron-sized cavities made of gold atop an insulating layer and a semiconductor material based on indium and antimony. The cavities trap photons between the gold and semiconductor layers, and surface plasmons – collective, coherent oscillations of conduction electrons that interact very strongly with light – then keep them on the surface of the semiconductor.

Working with scientists from the Collège de France and the Helmholtz-Zentrum Dresden-Rossendorf (HZDR) in Germany, the researchers applied pulses of THz light from the TELBE light source at the HZDR’s ELBE accelerator to their structure. They found that they could use this intense multi-cycle THz light field to modulate the material’s optical properties over timescales of just picoseconds.

Towards new types of lasers in the THz range

“This study builds on previous work in my group related to the development and study of tuneable plasmonic metamaterials in the THz range as a means to create functional devices to control light-matter interactions in this range,” Laplace says. “One of the central questions in our work was to determine if the temporal modulation of the metamaterial would be strong and fast enough.

“By developing a theoretical model in collaboration with our colleague Marco Schiró and his team at the Collège de France that reproduced the experimental observations remarkably well, we showed that the system presented the characteristic spectroscopic signatures expected for a PhTC and provided an explanation for the behaviour of the photons therein.”

The researchers, who detail their work in Nature, also found that the ultrafast temporal modulation reduced the dissipation of photons within the metamaterial by half and they are now looking to reduce these optical losses even further.

“The THz frequency range lies at the junction between electronic and photonic technologies and is historically less developed than these two,” Laplace explains. “With the THz PhTCs that are now achievable, we hope we can soon develop devices like THz amplifiers, frequency converters and maybe new types of THz lasers in this range, hence contributing to the closing of the so-called ‘THz gap,’” he tells Physics World.

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As the world of quantum computing grows and researchers work towards scaling up quantum systems, energy consumption is becoming a major concern. Beyond the small scale and high level of control in a laboratory environment, the lasers that power quantum systems result in a large energy cost that may act as a bottleneck for the integration of quantum technology.

Publishing their findings in Optica, researchers have demonstrated that sunlight can be used to generate pairs of entangled photons, providing a more energy efficient alternative to laser-pumped systems. This collaborative project combined theoretical research led by Robert Boyd at the University of Ottawa with technology developed by Hanieh Fattahi’s research group at the Max Plank Institute for the Science of Light in Erlangen, Germany.

Overcoming assumptions

Optical quantum computers use pairs of entangled photons as qubits, with the nonlinear optical processes used to produce them typically relying on lasers. This is largely due to two assumptions: firstly, that high optical coherence is required, meaning that the light waves maintain a steady phase relationship; and secondly, that lasers are the only way to achieve the necessary optical power density for these methods.

Sunlight, while naturally abundant, is largely incoherent and is difficult to collect in concentrations comparable to that of lasers. As such, this natural reservoir of optical input has been largely overlooked as a direct resource for nonlinear optical processes.

The researchers behind this latest study are challenging these assumptions with a new system that uses sunlight to fuel a process called spontaneous parametric down-conversion (SPDC). In this process, a pump beam – usually a laser but replaced here with solar light – interacts with a nonlinear crystal, splitting individual photons into entangled pairs.

Previous work from Boyd’s team demonstrated that incoherent light from an LED can produce photons with entangled polarization states. By achieving entanglement powered by sunlight, this new research further overturns both assumptions about the necessary properties of the optical input.

Harnessing the Sun

To harness the plentiful yet highly dispersed sunlight, Fattahi’s team had to develop a device that focuses sunlight down to a point approximately 2 mm wide, to be coupled to a fibre as thin as a human hair. To achieve this, they used a Fresnel lens and spectral filter to collect sunlight, and a glass cone-shaped concentrator to funnel the light to a point, where it is coupled to the fibre. The fibre then directs the sunlight into the nonlinear crystal to induce SPDC.

Fattahi described the “significant practical challenges” involved with implementing such a system. Along with having to continuously track the Sun, the outdoor nature of the experiment left it vulnerable to both environmental effects and background light. Eventually compensated for by enclosing the system in a tent, the background light was initially offset by students beginning measurements at around 3 a.m. to make the most of the natural darkness.

Overcoming both theoretical and practical concerns, the system was able to successfully produce entangled photons. The states produced violate Bell’s inequality (as the photon correlations cannot be modelled classically) with an S value of 2.54, where S = 2 is the threshold for indication of quantum behaviour, and a 94% fidelity to the target entangled Bell state.

Significantly, when normalized in terms of the spectral bandwidth of the pump, sunlight-powered SPDC demonstrates a photon pair generation rate comparable to that of the laser-pumped process. This method eliminates the need for electrical-to-optical energy conversion, providing a viable path towards increasing energy efficiency.

The future of photon production

The development of quantum technology is vital for the future of secure communication, ultraprecise sensing and high-performance computation. Taking steps to develop a sunlight-driven method of photon pair production will potentially allow scaling of this technology without the major energy cost.

Minimizing energy consumption and system complexity would be a huge benefit for systems operating in demanding conditions, such as polar deserts. This research is particularly striking when considering space-based quantum technology. Sun-synchronous orbits could allow near constant access to a naturally occurring, reliable pump-source.

Fattahi and her team intend to develop a field-deployable version of this system, with a focus on greater integration which should “significantly improve mechanical stability, efficiency and overall practicality”. There is also potential to expand the portion of the solar spectrum used in this experiment. Fattahi described the “exciting possibility” of using different spectral regions to drive multichannel entangled-photon generation, increasing efficiency and capacity.

Research into new, energy-efficient photon production has the potential to remove a major barrier for the integration of quantum technologies and contribute to a brighter future for quantum computing.

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Producing pairs of correlated or entangled photons usually requires a complex laser system. Now, however, researchers at China’s Xiamen University have shown that these crucial ingredients in quantum optics experiments can come from a far more basic source: sunlight. The discovery could simplify optical systems that rely on a process known as spontaneous parametric down-conversion (SPDC), allowing the technology to be deployed in space and other locations with limited or no access to electricity.

SPDC occurs when a short-wavelength photon passes through a nonlinear crystal and gets converted into twin photons with a longer wavelength. Traditionally, the initiating (pump) photon in this paired-photon source comes from a coherent laser. However, recent research suggested that fully coherent light sources might not be strictly necessary, and that partially coherent sources might also be able to drive SPDC.

A Sun-tracking system

In the new work, researchers led by Wuhong Zhang and Lixiang Chen took this idea even further. Could sunlight – which is inherently incoherent – also drive SPDC?

In principle, Zhang and Chen suspected the answer was “yes”. After all, a ray of sunlight, like a laser beam, is just a stream of photons. The problem is that unlike photons from a laser, the brightness and incidence angle of solar photons is constantly changing. This makes it difficult to collect enough pump photons to produce correlated photon pairs at high rates.

To overcome this problem, the researchers installed a Sun-tracking system on the roof of their laboratory building. This was essentially a telescope mount that moves with the Sun to collect light continuously throughout the day. They then worked out how to efficiently couple this collected sunlight into a multi-mode fibre and transmit it into their laboratory. There, they used the light to pump a nonlinear crystal made of periodically poled potassium titanyl phosphate (PPKTP). Within this crystal, the SPDC process converted pump photons into correlated photon pairs, demonstrating that it is indeed possible to use sunlight to generate photon pairs with strong position correlations.

The team faced numerous challenges along the way. The low spatial coherence and temporal instability of sunlight needed to be mitigated, and the coupling into the fibre needed to be very efficient. However, Chen notes that sunlight does have one advantage over traditional laser sources. “Sunlight is inherently broadband in its spectrum, so it can precisely provide any favourable wavelength,” he says. “This means it could be adapted to diverse application scenarios.”

Towards laser-free and electricity-independent SPDC light sources

According to Zhang, the team’s work shows that laser-free and electricity-independent SPDC light sources are possible. Potential applications could include correlation-enhanced sensing in remote areas and space-based quantum key distribution and teleportation, and he tells Physics World that one of the team’s next goals is to test the system in outdoor environments.

Chen adds that the system, which is described in Advanced Photonics, could also become a platform for fundamental studies of how the coherence of light affects the photon-splitting process in SPDC. He and his colleagues are now focusing on improving the efficiency of their sunlight collection system; optimizing the design of their nonlinear crystal so that it is better adapted to the Sun’s broadband spectrum; and implementing advanced image reconstruction techniques such as compressed sensing. “We think that introducing AI technologies such as artificial neural networks and deep learning into such imaging systems will be a key priority in going forward,” Chen says. “They will inform us on how to exploit sunlight more efficiently to implement various advanced quantum information protocols.”

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