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Organic p-type cathode materials are promising for sustainable energy storage due to their abundance, environmental compatibility, and high operating voltages exceeding 3.5 V. However, their application is constrained by high...
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Finely modulating the Cs : Pb ratio of the top 1 nm of CsPbI₃ leads to strong surface dipoles that alter the work function by more than 2 eV, increasing the power conversion efficiency from ∼10% to ∼20% and critically affecting stability.
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